激光诱导热透镜效应——空间自相位调制的实验教学推广EXPERIMENTAL TEACHING PROMOTION OF LASER-INDUCED THERMAL LENSING EFFECT IN TWO-DIMENSIONAL MATERIALS: SPATIAL SELF-PHASE MODULATION
杨博,李洁,李一鸣,乔中华,唐嘉岐,鄢小卿,王槿,刘东奇,刘芳
摘要(Abstract):
本文将理论与实验结合,设计了一套基于空间自相位调制(Spatial Self-Phase Modulation,SSPM)探究激光诱导热透镜效应的教学装置,观察了SSPM衍射条纹的形成-畸变-稳定的动态过程;利用该装置验证了衍射环数与激光光强的线性依赖关系,并发现入射光强相同时,激光波长越靠近材料吸收峰衍射环环数越多;将实验教学场景从传统的NMP(N-甲基吡咯烷酮)试剂进一步推广到安全性更高的茶多酚-乙醇试剂和固体样品。该装置不仅推广了热透镜效应在实验教学中的应用,还有望为新材料热透镜效应研究提供重要的实验平台和参考。
关键词(KeyWords): 热透镜效应;热致非线性;二维材料;空间自相位调制
基金项目(Foundation): 南开大学2025年科研仪器实验技术研发项目(项目批准号:25NKSYJS05);; 国家重点研发计划(项目批准号:2023YFB3307700);; 航空科学基金(项目批准号:202400540S6002)
作者(Author): 杨博,李洁,李一鸣,乔中华,唐嘉岐,鄢小卿,王槿,刘东奇,刘芳
DOI: 10.27024/j.wlygc.2025.11.07.02
参考文献(References):
- [1] GORDON J P,LEITE R C C,MOORE R S,et al.Long-transient effects in lasers with inserted liquid samples[J].Journal of Applied Physics,1965,36(1):3-8.
- [2] JOHN R W.Laser measurement of optical absorption in liquids[J].Accounts of Chemical Research,1974,7(7):225-231.
- [3] GEIM A K,GRIGORIEVA I V.Van der waals heterostructures[J].Nature,2013,499(7459):419-425.
- [4] WANG Y N,TANG Y J,CHENG P H,et al.Distinguishing thermal lens effect from electronic third-order nonlinear self-phase modulation in liquid suspensions of 2D nanomaterials[J].Nanoscale,2017,9(10):3547-3554.
- [5] WU L M,YUAN X X,MA D T,et al.Recent advances of spatial self-phase modulation in 2D materials and passive photonic device applications[J].Small,2020,16(35):2002252.
- [6] BERNARDI M,PALUMMO M,GROSSMAN J C.Extraordinary sunlight absorption and one nanometer thick photovoltaics using two-dimensional monolayer materials[J].Nano Letters,2013,13(8):3664-3670.
- [7] ZHANG J D,YU X F,HAN W J,et al.Broadband spatial self-phasemodulation of black phosphorous[J].Optics Letters,2016,41(8):1704-1707.
- [8] LIAO Y L,SONG C M,XIANG Y J,et al.Recent advances in spatial self-phase modulation with 2D materials and its applications[J].Annalen Der Physik,2020,532(12):2000322.
- [9] HU L L,SUN F,ZHAO H,et al.Nonlinear optical response spatial self-phase modulation in MoTe2:Correlations between χ(3) and mobility or effective mass[J].Optics Letters,2019,44(21):5214-5217.
- [10] NABANITA S,SAGNIK B,SOUVIK B C,et al.Unraveling SSPM Phenomena in Type-II Dirac Semimetal NiTe2 for All-Optical Diodes and Switching Applications[J].Small,2025,21(31):2503235.
- [11] WU L M,FAN T J,WEI S R,et al.All-optical logic devices based on black arsenic-phosphorus with strong nonlinear optical response and high stability[J].Opto-Electronic Advances,2022,5(1):200046.
- [12] WU Y L,WU Q,SUN F,et al.Emergence of electron coherence and two-color all-optical switching in MoS2 based on spatial self-phase modulation[J].PNAS,2015,112(38):11800-11805.